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The totally aromatic structures of the aramid polymers give them exceptional heat and ame resistance, very high melting points (generally above their decomposition temperature, which are !500 C), ultrahigh strength, and better resistance to solvents, chemicals, and oxidizing agents compared to aliphatic polyamides. Kevlar has higher strength and modulus properties compared to Nomex. The para structure of the former gives a rodlike extendedchain structure that forms liquid crystal solutions. (Liquid crystal solutions are solutions in which there is a high degree of ordering of solute molecules; see Sec. 2-14g.) Polymer crystallization from liquid crystal solutions results in a highly oriented, extended-chain morphology in the bulk polymer, resulting in high strength and high modulus.

1970 s and 1980 s, the relative gap between mortgage rates and bond yields narrowed, and the two series moved together. Since 1970 or so, mortgage rates have adjusted fairly quickly to changes in other yields, as the table also indicates. As presented in the table on page 420, mortgage rates averaged far above corporate bond yields in the easy-money period of the 1940 s and also in the 1950 s. As yields rose in the 1960 s, the yield spread in favor of mortgages came down sharply, and in the 1970 s and 1980 s it was nearly eliminated. Indeed, at times in the 1970 s and 1980 s, seasoned corporate bond yields exceeded some mortgage yields, while new issue corporate bond yields were far above high-grade mortgage yields. This big change in yield relationship was one of the most significant changes in recent decades. Why should savings institutions insist on mortgages if they yield less than prime corporate bonds, much less if the expenses of a mortgage portfolio are taken into account Hence government agencies intervened to permit the mortgage market to tap the money market and the bond market. Because of this intervention, even the massive failures of savings and loan institutions at the end of the 1980 s had minimal impact on mortgage rates. Before the 1960 s, relative stability at a high level was characteristic of rates, such as mortgage rates, that involve large servicing costs and

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= FIGURE C-17

Aramid polymers are much more expensive than the aliphatic polyamides. The use of aramid polymers is limited to those applications that justify the high cost. The present U.S. market is about 20 million pounds per year. The applications are those where one needs very high ame resistance (clothing for re ghters and welders, welder s protective shield, upholstery and drapes), heat resistance (ironing board covers, insulation lm for electrical motors and transformers, aerospace and military), dimensional stability ( re hose, V- and conveyor belts), or strength and modulus (circuit boards, bulletproof vests, ber optic and power lines, ship mooring ropes, automobile tire cord, puncture-resistant bicycle tires).

Wallace Carothers and coworkers at DuPont synthesized aliphatic polyesters in the 1930s [Furukawa, 1998; Hounshell and Smith, 1988]. These had melting points below 100 C, which made them unsuitable for rber use. Carothers then turned successfully to polyamides, based on the theoretical consideration that amides melt higher than esters. Polyamides were the rst synthetic bers to be produced commercially. The polyester and polyamide research at DuPont had a major impact on all of polymer science. Carothers laid the foundation for much of our understanding of how to synthesize polymeric materials. Out of that work came other discoveries in the late 1930s, including neoprene, an elastomer produced from chloroprene, and Te on, produced from tetra uoroethylene. The initial commercial application for nylon 6/6 was women s hosiery, but this was short-lived with the intrusion of World War II. The entire nylon 6/6 production was allocated to the war effort in applications for parachutes, tire cord, sewing thread, and rope. The civilian applications for nylon products burst forth and expanded rapidly after the war. Carother s work not only secured the future of the DuPont chemical empire but launched the synthetic ber industry and changed the agricultural patterns of the Southern cotton states. Subsequent to the success of nylon, workers in the United Kingdom in the early 1950s achieved success in producing a polyester ber by using terephthalate as the acid component. Cotton, no longer King of Fibers, accounts for less than 25% of the U.S. ber market. Nylon, PET, and rayon (regenerated cellulose) account for the remainder.

THE UNITED STATES IN THE TWENTIETH CENTURY: 1946 1990

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